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A tie between Tyranitar and Charizard.
When I first played Blue as a child I was obsessed with Dragons.
Since I did not know ANYTHING about the Pokemon games when I started to Play, had not watched the manga or seen pictures or anything I chose Charmander because it was a lizard that breathed fire and though "THAT'S COOL!"
To me absolute delight hitting level 36 as a 8 year old boy and having my Bro transform into a fucking full-blown dragon gave me my first boner.
My love for Tyranitar came in Silver, since I could not get anyone to trade my Charizard over to me from Blue I was disappointed with losing a huge dragon like creature.
Out of nowhere a Larvitar appeared, for some reason at age 10 I thought he would turn into another dragon aswell and level him as much as I could.
After going for so long and him not leveling for ages I was about to give up when my Pupitar finally evolved into the Monster that is Tyranitar.
He became my main Pokemon for the next 300hrs I sunk into that game.
Both are my Bros, and Both are always in my team in Every gen since.