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Apart from the red Gyarados, my first was a Nidorino in Pokémon Crystal, route 13, but it was in my GBC, so I don't have it anymore.
In the same save file I accidentally killed a shiny Venonat too.
Also, this is my shiny box, almost everything I could gather in my DS/3DS games, except for a Dragonite that I use in Alpha Sapphire and a Sneasel that I have no idea where it is.
Of course, the legendary Pokémon and Beldum came from events and Gyarados and Haxorus were 100% shiny (SoulSilver and White 2).