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My unexpected bro was my Luxray in Platinum. I caught him just because I wanted an electric type to go with my Piplup. Then as he evolved I started going, "Oh shit where's this going ofukofukofuk." Then he turned into some badass thunder lion and never failed me when I needed him. In fact, I always paired him with Empoleon in npc doubles and had them in the first two slots.
My unexpected bro also became pokebros with Penguimon.
His name is "Simbalol".
