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Banette.
I really like that they're driven by a grudge rather than a desire to just be a creepy shit.
Something I wonder though, would they turn back into a doll if they were to forgive their original owner, or would they stay a Banette?
Golurk comes into a close second, since they're kind of the "good guys" of ghost types. They are protectors. And like most people who like Golurk and even those who don't, it reminds me of the Iron Giant.