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My favorite overall Pokemon is Gen 5 and 2 Pokemon from Gen 4 round out my top 3, as a collective whole I'd rank them...
1=3>2=5>6>4>7
Yes, I may be blinded by nostalgia, but I like the most designs from Gen 1 and 3. Gen 7, though ranked last, still have some pretty killer designs.
If I actually had the autism to go through each gen, the rankings might actually be different.