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To address OP's deliberately chosen image, I missed old Takecha.
To the question, Entei is always a good pick for how straight to the point it is, even if Shudo's hoped for father/daughter angle is only just there. Mewtwo stumbles in the second half, I appreciate Lugia as spectacle movie pretty unabashedly now, never liked Latios/Latias... I think I need to revisit Deoxys and watch Darkrai, as I never have and I know people like it. I like Giratina, Arceus, and Zoroark but can't call them best.
