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I really like Unison and Marine Shukkou for the "expressing themselves in relation to their fans" part. Unison exposes all of her insecurities and her desperate need for validation, and how she gets it from her audience, and Shukkou feels like a search for drive and inspiration after the high ends, when you can no longer coast on the positive fluffy feelings that just being around Hololive gives you. Love these songs to bits.
>幸せは願えば手に入るほど安くはない
Her most underrated song, in my opinion. It's by the Sakura Wars composer, too, a dream come true for her.