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Call Me Tonight - while it might not seem so just from reading the synopsis, this is a work of legit genre subversion.
The Legend of Black Heaven - you can never really tell how delusional the main character is.
Alien Nine - mindfuck Pokemon.
And ignore the Aquarion autist. The shows he recommends are not necessarily bad, but he ignores the OP prompts entirely. For example, Giant Gorg is a great anime, but it's also a very straightforward adventure story, so it's like the opposite of what you're looking for.
