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Dancouga is amazing, but honestly not much of a combiner. He puts "boots" and a head on, and you're set. The base Big Moth's articulation sis o nice it makes it a great figure no matter what, but it does lose some wow factor you should get from combiners.
I really like SoC GoLion/Voltron and GaoGaiGar. I get thatVoltron lacks a certain "wow" factor since its so basic, but in hand it feels very nice, and compared to other combining robots it has the weight and height give it a commanding presence. Personally I'm glad they didn't hide the lion legs, I like the look with them exposed.
GaoGaiGar is great, and I think looks best just alone, free from all the expansion sets. I do own and display them all, having it with the StarGaoGaiGar upgrade, but you're best off with just the base figure.
Daizyujin/Megazord is a fun, but very underwhelming piece. Especially for th eprice. Like GGG, I don't think any expansions(Dragonzord & Titanus) would really improve the base figure since it'd just make it a brick, except for the alternate Dragonzord combo.
Gunbuster is another cool piece, but severely dated. It doesn't capture the animation look perfectly, but does an admirable job. Its a bit awkward due to weight distribution.
I'm inteerested in more, but aesthetically a lot of SoC releases are a bit too dated looking for me. When it comes to 70's/80's mecha, I usually prefer more dynamic redesigns,which is why Sentinel's Dancouga and their Obari line is up my alley.
Also interested in Generation Toy's Yellow gravity Builder, or G2 devastator. Their basic release doesn't match my G1 collection, but my G2 stuff is more a free-for-all