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I put Unova up there because of all the bumfuck nowhere locales like Anville, Lacunosa and Lentimas, lots of entire places out of the way that have no relevance to the Pokemon League or anything major in lore.
However, I put Unova on the top solely because of Village Bridge. Fuck, I love that place, a true 'mood' of a place. I'd pay good money to see it as part of one of the animated series or some prototype artwork to see tens of houses up there like a proper main road town.